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Comparison of measurement techniques for temperature and soot concentration in premixed, small-scale burner flames
Umeå universitet, Teknisk-naturvetenskapliga fakulteten, Institutionen för tillämpad fysik och elektronik. (Applied Laser Spectroscopy, TEC-Lab)
Umeå universitet, Teknisk-naturvetenskapliga fakulteten, Institutionen för tillämpad fysik och elektronik. (Applied Laser Spectroscopy, TEC-Lab)ORCID-id: 0000-0002-5065-7786
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2017 (Engelska)Ingår i: Energy & Fuels, ISSN 0887-0624, E-ISSN 1520-5029, Vol. 31, nr 10, s. 11328-11336Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Optical and intrusive measurement techniques for temperature and soot concentration in hot reacting flows were tested on a small-scale burner in fuel-rich, oxygen-enriched atmospheric flat flames produced to simulate the environment inside an entrained flow reactor. The optical techniques comprised two-color pyrometry (2C-PYR), laser extinction (LE), and tunable diode laser absorption spectroscopy (TDLAS), and the intrusive methods included fine-wire thermocouple thermometry (TC) and electrical low pressure impactor (ELPI) particle analysis. Vertical profiles of temperature and soot concentration were recorded in flames with different equivalence and O2/N2 ratios. The 2C-PYR and LE data were derived assuming mature soot. Gas temperatures up to 2200 K and soot concentrations up to 3 ppmv were measured. Close to the burner surface, the temperatures obtained with the pyrometer were up to 300 K higher than those measured by TDLAS. Further away from the burner, the difference was within 100 K. The TC-derived temperatures were within 100 K from the TDLAS results for most of the flames. At high signal-to-noise ratio and in flame regions with mature soot, the temperatures measured by 2C-PYR and TDLAS were similar. The soot concentrations determined with 2C-PYR were close to those obtained with LE but lower than the ELPI results. It is concluded that the three optical techniques have good potential for process control applications in combustion and gasification processes. 2C-PYR offers simpler installation and 2D imaging, whereas TDLAS and LE provide better accuracy and dynamic range without calibration procedures.

Ort, förlag, år, upplaga, sidor
Washington: American Chemical Society (ACS), 2017. Vol. 31, nr 10, s. 11328-11336
Nyckelord [en]
flow coal gasifier, volume fraction, wavelength dependence, optical diagnostics, refractive index, gas temperature, pyrometry, biomass, size, extinction
Nationell ämneskategori
Atom- och molekylfysik och optik Energisystem Kemiska processer
Identifikatorer
URN: urn:nbn:se:umu:diva-141034DOI: 10.1021/acs.energyfuels.7b01168ISI: 000413710300104OAI: oai:DiVA.org:umu-141034DiVA, id: diva2:1151103
Tillgänglig från: 2017-10-22 Skapad: 2017-10-22 Senast uppdaterad: 2018-06-09Bibliografiskt granskad

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Qu, ZhechaoSchmidt, Florian M.

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Energy & Fuels
Atom- och molekylfysik och optikEnergisystemKemiska processer

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