Umeå universitets logga

umu.sePublikationer
Ändra sökning
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf
Emerging Carbon-Based Heterogeneous Catalysts for Electrochemical Reduction of Carbon Dioxide into Value-Added Chemicals
Umeå universitet, Teknisk-naturvetenskapliga fakulteten, Institutionen för fysik. Department of Materials Science and NanoEngineering, Rice University, Houston, TX 77005, USA.
Visa övriga samt affilieringar
2019 (Engelska)Ingår i: Advanced Materials, ISSN 0935-9648, E-ISSN 1521-4095, Vol. 31, nr 13, artikel-id 1804257Artikel, forskningsöversikt (Refereegranskat) Published
Abstract [en]

The electrocatalytic reduction of CO2 provides a sustainable way to mitigate CO2 emissions, as well as store intermittent electrical energy into chemicals. However, its slow kinetics and the lack of ability to control the products of the reaction inhibit its industrial applications. In addition, the immature mechanistic understanding of the reduction process makes it difficult to develop a selective, scalable, and stable electrocatalyst. Carbon-based materials are widely considered as a stable and abundant alternative to metals for catalyzing some of the key electrochemical reactions, including the CO2 reduction reaction. In this context, recent research advances in the development of heterogeneous nanostructured carbon-based catalysts for electrochemical reduction of CO2 are summarized. The leading factors for consideration in carbon-based catalyst research are discussed by analyzing the main challenges faced by electrochemical reduction of CO2. Then the emerging metal-free doped carbon and aromatic N-heterocycle catalysts for electrochemical reduction of CO2 with an emphasis on the formation of multicarbon hydrocarbons and oxygenates are discussed. Following that, the recent progress in metal-nitrogen-carbon structures as an extension of carbon-based catalysts is scrutinized. Finally, an outlook for the future development of catalysts as well as the whole electrochemical system for CO2 reduction is provided.

Ort, förlag, år, upplaga, sidor
2019. Vol. 31, nr 13, artikel-id 1804257
Nyckelord [en]
aromatic N-heterocycles, carbon, CO2 reduction, heteroatom doping, metal-nitrogen-carbon ructures
Nationell ämneskategori
Fysikalisk kemi Den kondenserade materiens fysik
Identifikatorer
URN: urn:nbn:se:umu:diva-158381DOI: 10.1002/adma.201804257ISI: 000463970200006PubMedID: 30589109Scopus ID: 2-s2.0-85059134052OAI: oai:DiVA.org:umu-158381DiVA, id: diva2:1307649
Tillgänglig från: 2019-04-29 Skapad: 2019-04-29 Senast uppdaterad: 2023-03-23Bibliografiskt granskad

Open Access i DiVA

Fulltext saknas i DiVA

Övriga länkar

Förlagets fulltextPubMedScopus

Person

Sharifi, Tiva

Sök vidare i DiVA

Av författaren/redaktören
Sharifi, Tiva
Av organisationen
Institutionen för fysik
I samma tidskrift
Advanced Materials
Fysikalisk kemiDen kondenserade materiens fysik

Sök vidare utanför DiVA

GoogleGoogle Scholar

doi
pubmed
urn-nbn

Altmetricpoäng

doi
pubmed
urn-nbn
Totalt: 88 träffar
RefereraExporteraLänk till posten
Permanent länk

Direktlänk
Referera
Referensformat
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Annat format
Fler format
Språk
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Annat språk
Fler språk
Utmatningsformat
  • html
  • text
  • asciidoc
  • rtf