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Chemoenzymatic Dynamic Kinetic Resolution of Primary Benzylic Amines using Pd-0-CalB CLEA as a Biohybrid Catalyst
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2019 (engelsk)Inngår i: Chemistry - A European Journal, ISSN 0947-6539, E-ISSN 1521-3765, Vol. 25, nr 39, s. 9174-9179Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Herein, we report on the use a biohybrid catalyst consisting of palladium nanoparticles immobilized on cross-linked enzyme aggregates of lipase B of Candida antarctica (CalB CLEA) for the dynamic kinetic resolution (DKR) of benzylic amines. A set of amines were demonstrated to undergo an efficient DKR and the recyclability of the catalysts was studied. Extensive efforts to further elucidate the structure of the catalyst are presented.

sted, utgiver, år, opplag, sider
WILEY-V C H VERLAG GMBH , 2019. Vol. 25, nr 39, s. 9174-9179
Emneord [en]
amides, biohybrid catalysts, dynamic kinetic resolution, heterogeneous catalysis, key cross-linked zyme aggregates
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Identifikatorer
URN: urn:nbn:se:umu:diva-162000DOI: 10.1002/chem.201901418ISI: 000475680200007PubMedID: 31050831OAI: oai:DiVA.org:umu-162000DiVA, id: diva2:1342224
Tilgjengelig fra: 2019-08-13 Laget: 2019-08-13 Sist oppdatert: 2019-08-13bibliografisk kontrollert

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