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Structural insights into [Co4O4(C5H5N)(4)(CH3CO2)(4)](+), a rare Co(IV)-containing cuboidal complex
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2013 (English)In: Polyhedron, ISSN 0277-5387, E-ISSN 1873-3719, Vol. 64, no SI, p. 304-307Article in journal (Refereed) Published
Abstract [en]

We report high-frequency (up to 219 GHz) and correspondingly high-field electron paramagnetic resonance spectra and X-ray crystal structure of [Co4O4(pyridine)(4)(acetate)(4)](+) ([Co4O4(py)(4)(OAc)(4)](+)) that serves as a structural and spectroscopic model of cobalt-oxide films that are capable of oxidizing water. These results are, in large part, consistent with those from our earlier, lower-frequency study and serve to benchmark future high-field studies on paramagnetic states of the catalyst film. (C) 2013 Published by Elsevier Ltd.

Place, publisher, year, edition, pages
2013. Vol. 64, no SI, p. 304-307
Keyword [en]
Cobalt; EPR; Water-oxidation
National Category
Inorganic Chemistry Theoretical Chemistry
Identifiers
URN: urn:nbn:se:umu:diva-129117DOI: 10.1016/j.poly.2013.05.038OAI: oai:DiVA.org:umu-129117DiVA, id: diva2:1058629
Available from: 2016-12-21 Created: 2016-12-21 Last updated: 2018-06-09

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Ohlin, C. Andre

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