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Capping Efficiency of Various Carbonaceous and Mineral Materials for In Situ Remediation of Polychlorinated Dibenzo-p-dioxin and Dibenzofuran Contaminated Marine Sediments: Sediment-to-Water Fluxes and Bioaccumulation in Boxcosm Tests
Umeå University, Faculty of Science and Technology, Department of Chemistry.
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2012 (English)In: Environmental Science and Technology, ISSN 0013-936X, E-ISSN 1520-5851, Vol. 46, no 6, 3343-3351 p.Article in journal (Refereed) Published
Abstract [en]

The efficiency of thin-layer capping in reducing sediment-to-water fluxes and bioaccumulation of polychlorinated dibenzo-p-dioxins and dibenzofurans, hexachlorobenzene, and octachlorostyrene was investigated in a boxcosm experiment. The influence of cap thickness (0.5-5 cm) and different cap materials was tested using a three-factor experimental design. The cap materials consisted of a passive material (coarse or fine limestone or a marine clay) and an active material (activated carbon (AC) or kraft lignin) to sequester the contaminants. The cap thickness and the type of active material were significant factors, whereas no statistically significant effects of the type of passive material were observed. Sediment-to-water fluxes and bioaccumulation by the two test species, the surface-dwelling Nassarius nitidus and the deep-burrowing Nereis spp., decreased with increased cap thickness and with addition of active material. Activated carbon was more efficient than lignin, and a ∼90% reduction of fluxes and bioaccumulation was achieved with 3 cm caps with 3.3% AC. Small increases in fluxes with increased survival of Nereis spp. indicated that bioturbation by Nereis spp. affected the fluxes.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2012. Vol. 46, no 6, 3343-3351 p.
Keyword [en]
sediment-to-water fluxes, benthic bioaccumulation, thin-layer capping, cap thickness
National Category
Chemical Sciences
URN: urn:nbn:se:umu:diva-53343DOI: 10.1021/es203528vPubMedID: 22339559OAI: diva2:511622
Available from: 2012-03-22 Created: 2012-03-22 Last updated: 2012-04-17Bibliographically approved

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Josefsson, SarahWiberg, Karin
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