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Reflections on substrate water and dioxygen formation
Max-Planck-Institut für Chemische Energiekonversion, Mülheim an der Ruhr, Germany.
Umeå University, Faculty of Science and Technology, Department of Chemistry.
2013 (English)In: Biochimica et Biophysica Acta - Bioenergetics, ISSN 0005-2728, E-ISSN 1879-2650, Vol. 1827, no 8-9, 1020-1030 p.Article, review/survey (Refereed) Published
Abstract [en]

This brief article aims at presenting a concise summary of all experimental findings regarding substrate water-binding to the Mn4CaO5 cluster in photosystem II. Mass spectrometric and spectroscopic results are interpreted in light of recent structural information of the water oxidizing complex (WOC) obtained by x-ray crystallography, spectroscopy and theoretical modeling. Within this framework current proposals for the mechanism of photosynthetic water-oxidation are evaluated.

Place, publisher, year, edition, pages
Elsevier, 2013. Vol. 1827, no 8-9, 1020-1030 p.
Keyword [en]
Photosystem II, substrate water binding, mechanism of water oxidation, mechanism of oxygen evolution, water oxidizing complex (WOC), oxygen evolving complex (OEC), Mn4CaO5 cluster
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:umu:diva-65083DOI: 10.1016/j.bbabio.2013.01.013ISI: 000322414300013OAI: oai:DiVA.org:umu-65083DiVA: diva2:603293
Note

Special Issue: Metals in Bioenergetics and Biomimetics Systems

Available from: 2013-02-05 Created: 2013-02-05 Last updated: 2017-12-06Bibliographically approved

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CiteExportLink to record
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