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Modeling the downward transport of Pb-210 in Peatlands: Initial Penetration-Constant Rate of Supply (IP-CRS) model
Umeå University, Faculty of Science and Technology, Department of Ecology and Environmental Sciences.
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2016 (English)In: Science of the Total Environment, ISSN 0048-9697, E-ISSN 1879-1026, Vol. 541, 1222-1231 p.Article in journal (Refereed) PublishedText
Abstract [en]

The vertical distribution of 210Pb is commonly used to date peat deposits accumulated over the last 100-150 years. However, several studies have questioned this method because of an apparent post-depositional mobility of 210Pb within somepeat profiles. In this study, we introduce the Initial Penetration-Constant Rate of Supply (IP-CRS) model for calculating ages derived from 210Pb profiles that are altered by an initial migration of the radio-nuclide. This new, two-phased, model describes the distribution of atmospheric-derived 210Pb (210Pbxs) in peat taking into account both incorporation of 210Pb into the accumulating peat matrix as well as an initial flushing of 210Pb through the uppermost peat layers. The validity of the IP-CRS model is tested in four anomalous 210Pb peat records that showed some deviations from the typical exponential decay profile not explained by variations in peat accumulation rates. Unlike the most commonly used210Pb-dating model (Constant Rate of Supply (CRS)), the IP-CRS model estimates peat accumulation rates consistent with typical growth rates for peatlands from the same areas. Confidence in the IP-CRS chronology is also provided by the good agreement with independent chronological markers (i.e. 241Am and 137Cs). Our results showed that the IP-CRS can provide chronologies from peat records where 210Pb mobility is evident, being a valuable tool for studies reconstructing past environmental changes using peat archives during the Anthropocene.

Place, publisher, year, edition, pages
Elsevier, 2016. Vol. 541, 1222-1231 p.
Keyword [en]
Am-241, Cs-137, Chronology, Lead, Americium, Caesium, Pb-210
National Category
Environmental Sciences
Identifiers
URN: urn:nbn:se:umu:diva-113714DOI: 10.1016/j.scitotenv.2015.09.131ISI: 000365289300125PubMedID: 26476062OAI: oai:DiVA.org:umu-113714DiVA: diva2:890091
Available from: 2015-12-30 Created: 2015-12-28 Last updated: 2015-12-30Bibliographically approved

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Olid, CarolinaKlaminder, Jonatan
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