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Wide-field imaging of gas-phase K species in biomass combustion using photofragmentation laser absorption imaging
Umeå University, Faculty of Science and Technology, Department of Applied Physics and Electronics.
Umeå University, Faculty of Science and Technology, Department of Applied Physics and Electronics.ORCID iD: 0000-0002-5065-7786
2025 (English)In: Fuel, ISSN 0016-2361, E-ISSN 1873-7153, Vol. 381, no Part B, article id 133429Article in journal (Refereed) Published
Abstract [en]

Potassium (K) plays a key role in biomass combustion as its presence in the gas phase may lead to slagging, agglomeration and corrosion. To facilitate feedstock flexibility, a detailed understanding of the K chemistry during solid fuel conversion is needed. Here, we present photofragmentation laser absorption imaging for simultaneous, quantitative wide-field imaging of gaseous atomic K, potassium hydroxide (KOH) and potassium chloride (KCl) using a high-speed camera. Concentration images of the K species, at levels down to below parts-per-million, were acquired in a physical domain of 3.8-by-16.4 mm with a spatial resolution of 0.13 mm and a temporal resolution of 0.5 s after averaging. The technique was applied for imaging of the K species release from solid coffee husk and wheat straw samples combusted in a laboratory flame. Conversion of KCl salt was investigated as a reference. Significant differences in K species concentration and spatial distribution were observed between the fuels and between the devolatilization and char conversion stages. We also demonstrate spatial mapping of the atomic K fragment recombination rates with 1.2 µs time resolution, which constitutes a step towards reaction kinetics imaging.

Place, publisher, year, edition, pages
Elsevier, 2025. Vol. 381, no Part B, article id 133429
Keywords [en]
Biomass combustion, Laser absorption imaging, Photofragmentation, Potassium (K)
National Category
Atom and Molecular Physics and Optics Chemical Engineering Energy Engineering
Identifiers
URN: urn:nbn:se:umu:diva-231327DOI: 10.1016/j.fuel.2024.133429ISI: 001346823100001Scopus ID: 2-s2.0-85207075431OAI: oai:DiVA.org:umu-231327DiVA, id: diva2:1911631
Funder
Swedish Energy Agency, 36160-1The Kempe Foundations, JCK-2025The Kempe Foundations, JCK-1316Available from: 2024-11-08 Created: 2024-11-08 Last updated: 2025-02-18Bibliographically approved

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Thorin, EmilSchmidt, Florian

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