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Bridging physics-based and equivalent circuit models for lithium-ion batteries
Department of Electrical Engineering, Division of Electric Power Engineering, Chalmers University of Technology, Göteborg, Sweden.
Umeå University, Faculty of Science and Technology, Department of Mathematics and Mathematical Statistics.
Scania CV AB, Södertälje, Sweden.
Department of Chemistry – Ångström Laboratory, Uppsala University, Box 538, 75121, Uppsala, Sweden.
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2021 (English)In: Electrochimica Acta, ISSN 0013-4686, E-ISSN 1873-3859, Vol. 372, article id 137829Article in journal (Refereed) Published
Abstract [en]

In this article, a novel implementation of a widely used pseudo-two-dimensional (P2D) model for lithium-ion battery simulation is presented with a transmission line circuit structure. This implementation represents an interplay between physical and equivalent circuit models. The discharge processes of an LiNi0.33Mn0.33Co0.33O2-graphite lithium-ion battery under different currents are simulated, and it is seen the results from the circuit model agree well with the results obtained from a physical simulation carried out in COMSOL Multiphysics, including both terminal voltage and concentration distributions. Finally we demonstrated how the circuit model can contribute to the understanding of the cell electrochemistry, exemplified by an analysis of the overpotential contributions by various processes.

Place, publisher, year, edition, pages
Elsevier, 2021. Vol. 372, article id 137829
Keywords [en]
Lithium-ion battery, Overpotential, Pseudo-two-dimensional model, Transmission line model
National Category
Other Physics Topics
Identifiers
URN: urn:nbn:se:umu:diva-186317DOI: 10.1016/j.electacta.2021.137829ISI: 000619728100010Scopus ID: 2-s2.0-85100403454OAI: oai:DiVA.org:umu-186317DiVA, id: diva2:1581518
Funder
Swedish Energy Agency, P42789-1Available from: 2021-07-22 Created: 2021-07-22 Last updated: 2023-03-24Bibliographically approved

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Wang, Siyang

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