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Nanosecond photothermal effects in plasmonic nanostructures
Laboratory of Photonics and Microwave Engineering, School of Information and Communication Technology, KTH Royal Institute of Technology, Electrum 229, Kista, Sweden.
Laboratory of Photonics and Microwave Engineering, School of Information and Communication Technology, KTH Royal Institute of Technology, Electrum 229, Kista, Sweden.
Laboratory of Photonics and Microwave Engineering, School of Information and Communication Technology, KTH Royal Institute of Technology, Electrum 229, Kista, Sweden.
Laboratory of Photonics and Microwave Engineering, School of Information and Communication Technology, KTH Royal Institute of Technology, Electrum 229, Kista, Sweden; State Key Laboratory of Modern Optical Instrumentation, Department of Optical Engineering, Zhejiang University, Hangzhou, China.
2012 (Engelska)Ingår i: ACS Nano, ISSN 1936-0851, E-ISSN 1936-086X, Vol. 6, nr 3, s. 2550-2557Artikel i tidskrift (Refereegranskat) Published
Abstract [en]

Photothermal effects in plasmonic nanostructures have great potentials in applications for photothermal cancer therapy, optical storage, thermo-photovoltaics, etc. However, the transient temperature behavior of a nanoscale material system during an ultrafast photothermal process has rarely been accurately investigated. Here a heat transfer model is constructed to investigate the temporal and spatial variation of temperature in plasmonic gold nanostructures. First, as a benchmark scenario, we study the light-induced heating of a gold nanosphere in water and calculate the relaxation time of the nanosphere excited by a modulated light. Second, we investigate heating and reshaping of gold nanoparticles in a more complex metamaterial absorber structure induced by a nanosecond pulsed light. The model shows that the temperature of the gold nanoparticles can be raised from room temperature to >795 K in just a few nanoseconds with a low light luminance, owing to enhanced light absorption through strong plasmonic resonance. Such quantitative predication of temperature change, which is otherwise formidable to measure experimentally, can serve as an excellent guideline for designing devices for ultrafast photothermal applications.

Ort, förlag, år, upplaga, sidor
American Chemical Society (ACS), 2012. Vol. 6, nr 3, s. 2550-2557
Nyckelord [en]
thermodynamic, photothermal, metamaterial absorber
Nationell ämneskategori
Atom- och molekylfysik och optik
Identifikatorer
URN: urn:nbn:se:umu:diva-220541DOI: 10.1021/nn2050032ISI: 000301945900071Scopus ID: 2-s2.0-84859135597OAI: oai:DiVA.org:umu-220541DiVA, id: diva2:1834930
Tillgänglig från: 2024-02-06 Skapad: 2024-02-06 Senast uppdaterad: 2024-02-07Bibliografiskt granskad

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