Mid-infrared optical frequency comb spectroscopy using an all-silica antiresonant hollow-core fiberShow others and affiliations
2024 (English)In: Optics Express, E-ISSN 1094-4087, Vol. 32, no 6, p. 10679-10689
Article in journal (Refereed) Published
Abstract [en]
We present the first mid-infrared optical frequency comb spectrometer employing an absorption cell based on self-fabricated, all-silica antiresonant hollow-core fiber (ARHCF). The spectrometer is capable of measuring sub-mL sample volumes with 26 m interaction length and noise equivalent absorption sensitivity of 8.3 × 10−8 cm−1 Hz−1/2 per spectral element in the range of 2900 cm−1 to 3100 cm−1. Compared to a commercially available multipass cell, the ARHCF offers a similar interaction length in a 1000 times lower gas sample volume and a 2.8 dB lower transmission loss, resulting in better absorption sensitivity. The broad transmission windows of ARHCFs, in combination with a tunable optical frequency comb, make them ideal for multispecies detection, while the prospect of measuring samples in small volumes makes them a competitive technique to photoacoustic spectroscopy along with the robustness and prospect of coiling the ARHCFs open doors for miniaturization and out-of-laboratory applications.
Place, publisher, year, edition, pages
Optica Publishing Group , 2024. Vol. 32, no 6, p. 10679-10689
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:umu:diva-223068DOI: 10.1364/OE.517012Scopus ID: 2-s2.0-85187792371OAI: oai:DiVA.org:umu-223068DiVA, id: diva2:1852426
Funder
Knut and Alice Wallenberg Foundation, KAW 2020.0303Swedish Research Council, 2020-002382024-04-182024-04-182024-04-18Bibliographically approved