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Combined frequency comb and continuous wave cavity-enhanced optical-optical double-resonance spectrometer in the 1.7 µm range
Umeå University, Faculty of Science and Technology, Department of Physics.ORCID iD: 0000-0002-5627-1497
Umeå University, Faculty of Science and Technology, Department of Physics.ORCID iD: 0000-0001-6144-4957
Umeå University, Faculty of Science and Technology, Department of Physics.ORCID iD: 0000-0001-5790-2185
Umeå University, Faculty of Science and Technology, Department of Physics.
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2025 (English)In: Optics Express, E-ISSN 1094-4087, Vol. 33, no 18, p. 38776-38802Article in journal (Refereed) Published
Abstract [en]

We present an optical-optical double-resonance (OODR) spectrometer based on a 3.3 µm continuous wave pump and two cavity-enhanced probes: a frequency comb tunable in the 1.64–1.8 µm range, and a comb-referenced continuous wave (CW) laser tunable in the 1.6–1.75 µm range. The comb probe provides broad spectral coverage (bandwidth up to 7 THz) for simultaneous detection of many sub-Doppler OODR transitions with sub-MHz line position accuracy, while the CW probe allows targeting individual transitions with kHz accuracy and a higher signal-to-noise ratio in shorter time. Using the pump stabilized to the frequency of the R(0) transition in the v3 band of methane and the comb probe covering the 5550 to 6070 cm−1 interval, we detect 37 ladder-type transitions in the 3v3 ← v3 band region and 6 V-type transitions in the 2v3 band region and assign them using available theoretical predictions. Using the CW probe, we measure selected ladder- and V-type transitions with much higher precision. We also detect Lamb dips in the R(0) – R(3) transitions of the 2v3 band and report their center frequencies with kHz-level accuracy. The synergy effects of the comb- and CW-OODR open new possibilities in precision spectroscopy of levels that cannot be reached from the ground state.

Place, publisher, year, edition, pages
Optica Publishing Group, 2025. Vol. 33, no 18, p. 38776-38802
National Category
Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:umu:diva-245323DOI: 10.1364/OE.571448ISI: 001569342200003PubMedID: 40984278Scopus ID: 2-s2.0-105015576627OAI: oai:DiVA.org:umu-245323DiVA, id: diva2:2005432
Funder
Knut and Alice Wallenberg Foundation, KAW 2020.0303Swedish Research Council, 2020-00238Wenner-Gren Foundations, GFOv2024-0010Available from: 2025-10-09 Created: 2025-10-09 Last updated: 2025-10-09Bibliographically approved

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Silva de Oliveira, ViniciusHjältén, AdrianSilander, IsakRosina, AndreaFoltynowicz, Aleksandra

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