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Reaction mechanisms and catalysis in solar water splitting
Umeå University, Faculty of Science and Technology, Department of Physics.ORCID iD: 0009-0003-9618-3162
Umeå University, Faculty of Science and Technology, Department of Physics.
Umeå University, Faculty of Science and Technology, Department of Physics.
Umeå University, Faculty of Science and Technology, Department of Physics.ORCID iD: 0000-0001-9239-0541
2025 (English)In: Photon to power: harvesting the sun / [ed] Prasanth Ravindran; Deepa K. G.; Adersh Asok; Durga Shankar; Al Jumlat Ahmed, Singapore: Springer, 2025, p. 303-341Chapter in book (Refereed)
Abstract [en]

Solar water splitting, through electrocatalysis, photoelectrocatalysis, and photocatalysis, presents a promising pathway for converting abundant solar energy into clean hydrogen fuel. However, to meet the increasing demand for green hydrogen, catalysts for the water splitting reaction must not only achieve high efficiency but also be primarily composed of abundant materials with minimal environmental impact. Understanding the interplay between surface properties, optical properties, and chemical reactivity is crucial to identify suitable alternative materials capable of achieving high solar-to-hydrogen conversion. In this chapter, we discuss the fundamentals of electrochemical, photoelectrochemical, and photocatalytic water splitting. We explore how material’s properties and surface characteristics influence the hydrogen evolution reaction and oxygen evolution reaction. We revise their working principles and key concepts, from light absorption and charge separation to surface characteristics and adsorption energies. Additionally, we discuss key physical, chemical, and optical properties of electrodes and photoelectrodes that are crucial for an efficient water splitting, while presenting strategies for achieving high performance.

Place, publisher, year, edition, pages
Singapore: Springer, 2025. p. 303-341
Series
Progress in Optical Science and Photonics, ISSN 2363-5096, E-ISSN 2363-510X ; 32
Keywords [en]
Electrocatalysis, Hydrogen evolution, Oxygen evolution, Photocatalysis, Water electrolysis
National Category
Physical Chemistry Atom and Molecular Physics and Optics
Identifiers
URN: urn:nbn:se:umu:diva-246028DOI: 10.1007/978-981-96-5914-2_9Scopus ID: 2-s2.0-105019291759ISBN: 978-981-96-5913-5 (print)ISBN: 978-981-96-5916-6 (print)ISBN: 978-981-96-5914-2 (electronic)OAI: oai:DiVA.org:umu-246028DiVA, id: diva2:2010209
Available from: 2025-10-30 Created: 2025-10-30 Last updated: 2025-10-31Bibliographically approved

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Canto-Aguilar, Esdras J.Puentes-Prado, Laura ElenaKuzhikandathil Mohamed, AliceGracia-Espino, Eduardo

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Canto-Aguilar, Esdras J.Puentes-Prado, Laura ElenaKuzhikandathil Mohamed, AliceGracia-Espino, Eduardo
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Physical ChemistryAtom and Molecular Physics and Optics

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