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  • 1.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Boudon, Vincent
    Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS/Université Bourgogne Franche-Comté, 9 Av. A. Savary, BP 47870, Dijon Cedex, France.
    Richard, Cyril
    Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS/Université Bourgogne Franche-Comté, 9 Av. A. Savary, BP 47870, Dijon Cedex, France.
    Krzempek, Karol
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Hudzikowski, Arkadiusz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Głuszek, Aleksander
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Soboń, Grzegorz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    A methane line list with sub-MHz accuracy in the 1250 to 1380 cm−1 range from optical frequency comb Fourier transform spectroscopy2022In: Journal of Quantitative Spectroscopy and Radiative Transfer, ISSN 0022-4073, E-ISSN 1879-1352, Vol. 288, article id 108252Article in journal (Refereed)
    Abstract [en]

    We use a Fourier transform spectrometer based on a difference frequency generation optical frequency comb to measure high-resolution, low-pressure, room-temperature spectra of methane in the 1250 – 1380-cm−1 range. From these spectra, we retrieve line positions and intensities of 678 lines of two isotopologues: 157 lines from the 12CH4 ν4 fundamental band, 131 lines from the 13CH4 ν4 fundamental band, as well as 390 lines from two 12CH4 hot bands, ν2 + ν4 ν2 and 2ν4ν4. For another 165 lines from the 12CH4 ν4 fundamental band we retrieve line positions only. The uncertainties of the line positions range from 0.19 to 2.3 MHz, and their median value is reduced by a factor of 18 and 59 compared to the previously available data for the 12CH4 fundamental and hot bands, respectively, obtained from conventional FTIR absorption measurements. The new line positions are included in the global models of the spectrum of both methane isotopologues, and the fit residuals are reduced by a factor of 8 compared to previous absorption data, and 20 compared to emission data. The experimental line intensities have relative uncertainties in the range of 1.5 – 7.7%, similar to those in the previously available data; 235 new 12CH4 line intensities are included in the global model.

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  • 2.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Boudon, Vincent
    Laboratoire Interdisciplinaire Carnot de Bourgogne, Université Bourgogne Franche-Comté, Dijon, France.
    Richard, Cyril
    Laboratoire Interdisciplinaire Carnot de Bourgogne, Université Bourgogne Franche-Comté, Dijon, France.
    Krzempek, Karol
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Hudzikowski, Arkadiusz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Głuszek, Aleksander
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Soboń, Grzegorz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    An Accurate Methane Line List in the 7.2-8.0 µm Range from Comb-Based Fourier Transform Spectroscopy2022In: CLEO: 2022: Conference on Lasers and Electro-Optics, Optica Publishing Group , 2022, article id SM3F.6Conference paper (Refereed)
    Abstract [en]

    We use comb-based Fourier transform spectroscopy to record high-resolution spectra of 12CH4 and 13CH4 from 1250 to 1380 cm-1. We obtain line positions and intensities of 4 bands with uncertainties of ~450 kHz and ~3%, respectively, which we use to improve a global fit of the effective Hamiltonian.

  • 3.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Boudon, Vincent
    Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS, Université Bourgogne Franche-Comté, 9 Av. A. Savary, BP 47870, Dijon, France.
    Richard, Cyril
    Laboratoire Interdisciplinaire Carnot de Bourgogne, UMR 6303 CNRS, Université Bourgogne Franche-Comté, 9 Av. A. Savary, BP 47870, Dijon, France.
    Krzempek, Karol
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Hudzikowski, Arkadiusz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Głuszek, Aleksander
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Soboń, Grzegorz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wybrzeże Wyspiańskiego 27, Wrocław, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    An Accurate Methane Line List in the 7.2-8.0 μm Range from Comb-Based Fourier Transform Spectroscopy2022In: 2022 Conference on Lasers and Electro-Optics, CLEO 2022 - Proceedings, Optica Publishing Group , 2022, article id SM3F.6Conference paper (Refereed)
    Abstract [en]

    We use comb-based Fourier transform spectroscopy to record high-resolution spectra of 12CH4 and 13CH4 from 1250 to 1380 cm-1. We obtain line positions and intensities of 4 bands with uncertainties of ~450 kHz and ~3%, respectively, which we use to improve a global fit of the effective Hamiltonian.

  • 4.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Boudon, Vincent
    Laboratoire ICB, UMR 6303, CNRS, Université Bourgogne Franche-Comté, Dijon, France.
    Richard, Cyril
    Laboratoire ICB, UMR 6303, CNRS, Université Bourgogne Franche-Comté, Dijon, France.
    Tennyson, Jonathan
    Department of Physics and Astronomy, University College London, London, United Kingdom.
    Yurchenko, Sergey
    Department of Physics and Astronomy, University College London, London, United Kingdom.
    Gordon, Iouli E.
    Center for Astrophysics, Harvard & Smithsonian, Atomic and Molecular Physics Division, MA, Cambridge, United States.
    Pett, Christian
    Umeå University, Faculty of Science and Technology, Department of Chemistry.
    Silander, Isak
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Faculty of Electronics Photonics and Microsystems, Wrocław University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Faculty of Electronics Photonics and Microsystems, Wrocław University of Science and Technology, Wroclaw, Poland.
    Głuszek, Aleksander
    Faculty of Electronics Photonics and Microsystems, Wrocław University of Science and Technology, Wroclaw, Poland.
    Soboń, Grzegorz
    Faculty of Electronics Photonics and Microsystems, Wrocław University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    High accuracy line lists of CH4 and H2CO in the 8 µm range from optical frequency comb fourier transform spectroscopy2023In: 2023 conference on lasers and electro-optics Europe & European quantum electronics conference (CLEO/Europe-EQEC), IEEE, 2023, article id 10232703Conference paper (Refereed)
  • 5.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Gordon, Iouli E.
    Center for Astrophysics, Harvard & Smithsonian, Atomic and Molecular Physics Division, MA, Cambridge, United States.
    Tennyson, Jonathan
    Department of Physics and Astronomy, University College London, London, United Kingdom.
    Yurchenko, Sergey
    Department of Physics and Astronomy, University College London, London, United Kingdom.
    Krzempek, Karol
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Gluszek, Aleksander
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Pett, Christian
    Umeå University, Faculty of Science and Technology, Department of Chemistry.
    Silander, Isak
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Soboii, Grzegorz
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Precision frequency comb spectroscopy in the 8 µm range2023In: CLEO 2023: proceedings, Optical Society of America, 2023, article id AW4E.1Conference paper (Refereed)
    Abstract [en]

    We use Fourier transform spectroscopy based on a compact difference frequency generation comb source emitting around 8 μm to record broadband high-resolution spectra of molecules relevant to astrophysics and environmental monitoring. From the spectra we obtain line lists with sub-MHz accuracy, an order of magnitude better than previously available, and use them to refine theoretical models of these molecules. Here we report results for formaldehyde, for which the 8 μm range is missing in HITRAN.

  • 6.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser and Fiber Electronics Group, Faculty of Electronics, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Gluszek, Aleksander
    Laser and Fiber Electronics Group, Faculty of Electronics, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Tomaszewska, Dorota
    Laser and Fiber Electronics Group, Faculty of Electronics, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Sobon, Grzegorz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wroclaw University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Frequency comb fourier transform spectroscopy at 8 µm using a compact difference frequency generation source2021In: 2021 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC), IEEE, 2021Conference paper (Refereed)
  • 7.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Laser Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Gluszek, Aleksander
    Laser Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Tomaszewska, Dorota
    Laser Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Sobon, Grzegorz
    Laser Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Frequency Comb Fourier Transform Spectroscopy at 8m Using a Compact Difference Frequency Generation Source2021In: 2021 Conference on Lasers and Electro-Optics Europe and European Quantum Electronics Conference, CLEO/Europe-EQEC 2021, IEEE Lasers and Electro-Optics Society, 2021Conference paper (Refereed)
    Abstract [en]

    Mid-infrared comb-based Fourier transform spectroscopy allows high-resolution measurements of entire molecular absorption bands. However, most previous implementations were limited to wavelengths <5m. We present a Fourier transform spectrometer (FTS) with a comb-mode-limited resolution based on a compact difference frequency generation (DFG) source operating around 8m. We measure the spectrum of the ν 1 band of N 2 O in the Doppler limit and retrieve line center frequencies with precision of the order of 100 kHz.

  • 8.
    Germann, Matthias
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Tennyson, Jonathan
    Department of Physics and Astronomy, University College London, Gower Street, London, United Kingdom.
    Yurchenko, Sergei N.
    Department of Physics and Astronomy, University College London, Gower Street, London, United Kingdom.
    Gordon, Iouli E.
    Center for Astrophysics, Harvard & Smithsonian, Atomic and Molecular Physics Division, MA, Cambridge, United States.
    Pett, Christian
    Umeå University, Faculty of Science and Technology, Department of Chemistry.
    Silander, Isak
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Hudzikowski, Arkadiusz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Głuszek, Aleksander
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Soboń, Grzegorz
    Laser & Fiber Electronics Group, Faculty of Electronics, Photonics and Microsystems, Wrocław University of Science and Technology, Wrocław, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Optical frequency comb Fourier transform spectroscopy of formaldehyde in the 1250 to 1390 cm−1 range: experimental line list and improved MARVEL analysis2024In: Journal of Quantitative Spectroscopy and Radiative Transfer, ISSN 0022-4073, E-ISSN 1879-1352, Vol. 312, article id 108782Article in journal (Refereed)
    Abstract [en]

    We use optical frequency comb Fourier transform spectroscopy to record high-resolution, low-pressure, room-temperature spectra of formaldehyde (H212C16O) in the range of 1250 to 1390 cm−1. Through line-by-line fitting, we retrieve line positions and intensities of 747 rovibrational transitions: 558 from the ν6 band, 129 from the ν4 band, and 14 from the ν3 band, as well as 46 from four different hot bands. We incorporate the accurate and precise line positions (0.4 MHz median uncertainty) into the MARVEL (measured active vibration-rotation energy levels) analysis of the H2CO spectrum. This increases the number of MARVEL-predicted energy levels by 82 and of rovibrational transitions by 5382, and substantially reduces uncertainties of MARVEL-derived H2CO energy levels over a large range: from pure rotational levels below 200 cm−1 up to multiply excited vibrational levels at 6000 cm−1. This work is an important step toward filling the gaps in formaldehyde data in the HITRAN database.

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    fulltext
  • 9.
    Hjältén, Adrian
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Germann, Matthias
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser & Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Laser & Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Głuszek, Aleksander
    Laser & Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Tomaszewska, Dorota
    Laser & Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Soboń, Grzegorz
    Laser & Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Optical frequency comb Fourier transform spectroscopy of 14N216O at 7.8 µm2021In: Journal of Quantitative Spectroscopy and Radiative Transfer, ISSN 0022-4073, E-ISSN 1879-1352, Vol. 271, article id 107734Article in journal (Refereed)
    Abstract [en]

    We use a Fourier transform spectrometer based on a compact mid-infrared difference frequency generation comb source to perform broadband high-resolution measurements of nitrous oxide, 14N216O, and retrieve line center frequencies of the ν1 fundamental band and the ν1 + ν2 – ν2 hot band. The spectrum spans 90 cm−1 around 1285 cm−1 with a sample point spacing of 3 × 10−4 cm−1 (9 MHz). We report line positions of 72 lines in the ν1 fundamental band between P(37) and R(38), and 112 lines in the ν1 + ν2 – ν2 hot band (split into two components with e/f rotationless parity) between P(34) and R(33), with uncertainties in the range of 90-600 kHz. We derive upper state constants of both bands from a fit of the effective ro-vibrational Hamiltonian to the line center positions. For the fundamental band, we observe excellent agreement in the retrieved line positions and upper state constants with those reported in a recent study by AlSaif et al. using a comb-referenced quantum cascade laser [J Quant Spectrosc Radiat Transf, 2018;211:172-178]. We determine the origin of the hot band with precision one order of magnitude better than previous work based on FTIR measurements by Toth [http://mark4sun.jpl.nasa.gov/n2o.html], which is the source of the HITRAN2016 data for these bands.

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    fulltext
  • 10.
    Hjältén, Adrian
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Germann, Matthias
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Głuszek, Aleksander
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Tomaszewska, Dorota
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Soboń, Grzegorz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Precision measurements of 14N216O using a comb-based fourier transform spectrometer at 7.8 µm2021In: CLEO: Science and Innovations: Conference Proceedings, Optical Society of America, 2021, article id SM1C.4Conference paper (Refereed)
    Abstract [en]

    Using a compact fiber-based difference frequency generation comb and a Fourier transform spectrometer we record spectra of the N2O ν1 band at 1285 cm-1 in the Doppler limit. Fitting Gaussian line shapes to the individual absorption lines yields center frequencies with <200 kHz average precision.

  • 11.
    Hjältén, Adrian
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Germann, Matthias
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Sadiek, Ibrahim
    Leibniz Institute for Plasma Science and Technology (INP), Greifswald, Germany.
    Lu, Chuang
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Vieira, Francisco Senna
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Krzempek, Karol
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Głuszek, Aleksander
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Tomaszewska, Dorota
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Stuhr, Michael
    Institute of Physical Chemistry, University of Kiel, Kiel, Germany.
    Soboń, Grzegorz
    Laser and Fiber Electronics Group, Faculty of Electronics, Wrocław University of Science and Technology, Wroclaw, Poland.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Fourier transform spectroscopy using difference frequency generation comb sources at 3.3 µm and 7.8 µm2021In: Proceedings OSA Optical Sensors and Sensing Congress 2021 (AIS, FTS, HISE, SENSORS, ES), Optical Society of America, 2021, article id JTu4D.3Conference paper (Refereed)
    Abstract [en]

    We use offset-frequency-free difference frequency generation comb sources and a Fourier transform spectrometer with comb-mode-width limited resolution to measure and analyze spectra of molecular species of atmospheric relevance: CH3I and CH2Br2 around 3000 cm-1, and 14N216O around 1280 cm-1

  • 12.
    Hjältén, Adrian
    et al.
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Sadiek, Ibrahim
    Leibniz Institute for Plasma Science and Technology (INP), Greifswald, Germany.
    Lu, Chuang
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Vieira, Francisco Senna
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Stuhr, Michael
    Institute of Physical Chemistry, University of Kiel, Kiel, Germany.
    Germann, Matthias
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    High-Resolution Measurements of Halogenated Volatile Organic Compounds Using Frequency Comb Fourier Transform Spectroscopy2021In: 2021 Conference on Lasers and Electro-Optics Europe and European Quantum Electronics Conference, CLEO/Europe-EQEC 2021, IEEE Lasers and Electro-Optics Society, 2021Conference paper (Refereed)
    Abstract [en]

    Halogenated volatile organic compounds (HVOCs) play an important role in the photo-chemistry of the atmosphere, for example in ozone depletion [1]. They are produced naturally in the oceans but are also used in industrial and agricultural applications where they may pose a health-hazard due to their biological effects. Optical detection of these compounds would hence be of great value in, for example, atmospheric monitoring and leak detection in workplaces. Crucial for such detection schemes is access to accurate spectroscopic models, which in turn require high-precision laboratory measurements. Due to the combination of broad spectral coverage and high resolution, optical frequency comb Fourier transform spectroscopy is an excellent tool for providing the necessary spectroscopic data. We use a mid-infrared frequency comb and a Fourier transform spectrometer (FTS) to measure and assign high-resolution spectra of multiple absorption bands of two HVOCs: methyl iodide, CH 3 I [2] , and dibromomethane, CH 2 Br 2 , around 3.3m.

  • 13.
    Krzempek, Karol
    et al.
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Tomaszewska-Rolla, Dorota
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Gluszek, Aleksander
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Hudzikowski, Arkadiusz
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Krakowski, Mikolaj
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Hjältén, Adrian
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Germann, Matthias
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Foltynowicz, Aleksandra
    Umeå University, Faculty of Science and Technology, Department of Physics.
    Sobon, Grzegorz
    Faculty of Electronics, Photonics and Microsystems, Wroclaw University of Science and Technology, Wybrzeze Wyspianskiego 27, Wroclaw, Poland.
    Compact fiber-based mid-infrared frequency comb sources2022In: Optica High-brightness Sources and Light-driven Interactions Congress 2022, Optica Publishing Group (formerly OSA) , 2022, article id MW6C.1Conference paper (Refereed)
    Abstract [en]

    We report the development of compact, stabilized fiber-based mid-infrared frequency comb sources covering the 7–9 μm and 3.1–3.4 μm spectral ranges. Both sources enable high-precision Fourier-transform spectroscopy of greenhouse gases.

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